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Ngounié is one of Gabon's nine provinces. It covers an area of 37,750 km². The provincial capital is Mouila.

To the southeast, Ngounié borders the Niari Region of the Republic of the Congo. Domestically, it borders the following provinces:

   Nyanga - south

   Ogooué-Maritime - west

   Moyen-Ogooué - north

   Ogooué-Ivindo - northeast, at a quadripoint

   Ogooué-Lolo - east